Abstract:AlN buffer layers with various thicknesses were grown on sapphire substrates by pulsed laser deposition (PLD), and then GaN films were epitaxially grown. The crystalline quality and surface morphology of the as-grown GaN films were characterized by high-revolution X-ray diffraction (HRXRD) and scanning electron microscopy (SEM), respectively. It is found that GaN films grown with AlN buffer layer show a poorer crystalline quality but better surface morphology compared with GaN films without AlN buffer layer. Furthermore, when the AlN buffer layer thickness increases, both the crystalline quality and the surface morphology of GaN films are improved dramatically. In this regards, the thickness of AlN buffer layer plays an important role in achieving high crystalline quality and excellent surface morphology of GaN films.